Direct comparison of the in vitro and in vivo stability of DFO, DFO* and DFOcyclo* for Zr-immunoPET.

Fiche publication


Date publication

juin 2019

Journal

European journal of nuclear medicine and molecular imaging

Auteurs

Membres identifiés du Cancéropôle Est :
Pr DENAT Franck, Dr GONCALVES Victor


Tous les auteurs :
Raavé R, Sandker G, Adumeau P, Jacobsen CB, Mangin F, Meyer M, Moreau M, Bernhard C, Da Costa L, Dubois A, Goncalves V, Gustafsson M, Rijpkema M, Boerman O, Chambron JC, Heskamp S, Denat F

Résumé

Currently, the most commonly used chelator for labelling antibodies with Zr for immunoPET is desferrioxamine B (DFO). However, preclinical studies have shown that the limited in vivo stability of the Zr-DFO complex results in release of Zr, which accumulates in mineral bone. Here we report a novel chelator DFOcyclo*, a preorganized extended DFO derivative that enables octacoordination of the Zr radiometal. The aim was to compare the in vitro and in vivo stability of [Zr]Zr-DFOcyclo*, [Zr]Zr-DFO* and [Zr]Zr-DFO.

Mots clés

89Zr, DFO, DFO*, DFOcyclo*, Monoclonal antibodies, immunoPET

Référence

Eur. J. Nucl. Med. Mol. Imaging. 2019 Jun 3;: